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Journal Articles

Preliminary study of the criticality monitoring method based on the simulation for the activity ratio of short half-life noble-gas fission products from fuel debris

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo

Journal of Nuclear Science and Technology, 8 Pages, 2024/00

 Times Cited Count:0 Percentile:0.08(Nuclear Science & Technology)

Journal Articles

Depletion calculation of subcritical system with consideration of spontaneous fission reaction

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi

Journal of Nuclear Science and Technology, 59(4), p.424 - 430, 2022/04

 Times Cited Count:1 Percentile:15.7(Nuclear Science & Technology)

Journal Articles

Decay modes of heavy and superheavy nuclei

Koura, Hiroyuki

RIKEN Accelerator Progress Report, Vol.38, P. 9, 2005/05

We calculate proton-emission partial half lives and discuss dominant decay modes in the heavy and superheavy nuclidic region. The proton-emission partial half-lives are calculated from the one-dimensional WKB method with single-proton potentials and a mass formula that our group has developed. The calculated half lives well reproduce experimental ones in order of 100 or 1/100 which is similar predictability to other predictions as the alpha decay and the beta decay. We apply this result to calculation of branching ratios of nuclear decays considered the alpha decay, beta decay and spontaneous fission in the heavy and superheavy nuclide region. In this analysis we point out that proton-emitting nuclei are expected to be in the unknown proton-rich nuclidic region with $$N = 126$$. On the other hand, proton-rich nuclei with $$130 < N <160$$ have much shorter spontaneous-fission half-lives than ones of proton emissions on this calculation, therefore we conclude that ground-state proton emissions would not occur in that region.

Journal Articles

Gamma rays of short-lived ruthenium nuclides produced in the spontaneous fission of $$^{252}$$Cf

Shinohara, Nobuo; ; *; Tsukada, Kazuaki*; Otsuki, Tsutomu*; J.Alstad*

Radiochimica Acta, 56, p.127 - 131, 1992/00

no abstracts in English

Journal Articles

Measurement of the spontaneous fission half-life of $$^{242}$$Cm by absolute fission track counting

Usuda, Shigekazu; Umezawa, Hirokazu

Nucl. Tracks Radiat. Meas., 16(4), p.247 - 251, 1989/00

no abstracts in English

Oral presentation

Spontaneous fission measurements for nuclei around neutron-rich Fm region produced by using an $$^{254}$$Es target

Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.

no journal, , 

Spontaneous fissions of $$^{256}$$Fm, $$^{258}$$Fm, and $$^{259}$$Lr have been measured using an $$^{254}$$Es target at the JAEA Tandem Accelerator Facility. These three nuclei show different fission properties: the asymmetric fission, the high total-kinetic-energy (TKE) symmetric fission, and the low TKE symmetric fission, and the mechanisms of these three fissions should be very different. It is of great interest to elucidate how these differences occur. We have produced $$^{256,258}$$Fm in multinucleon-transfer reactions with a $$^{254}$$Es target and $$^{18}$$O projectiles, and produced $$^{259}$$Lr in the $$^{248}$$Cm($$^{15}$$N,4n) fusion-evaporation reaction. The reaction products were mass-separated with a gas-jet-coupled on-line isotope separator, and were delivered into a rotating wheel alpha- and fission-fragment detection system. By comparing the mass and TKE distributions deduced from the present experimental data, we will discuss the differences in fission mechanism among $$^{256}$$Fm, $$^{258}$$Fm, and $$^{259}$$Lr.

Oral presentation

Spontaneous fission measurements for neutron-rich Fm isotopes using an $$^{254}$$Es target

Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.

no journal, , 

Spontaneous fissions of neutron-rich heavy actinide isotopes $$^{256}$$Fm, $$^{258}$$Fm, and $$^{259}$$Lr have been measured at the JAEA Tandem accelerator facility. $$^{256}$$Fm and $$^{258}$$Fm were produced in a multinucleon transfer reaction with an $$^{18}$$O beam and an extremely rare $$^{254}$$Es target with a half-life of 276 days. Reaction products were mass-separated with an on-line isotope separator (ISOL). A transition between the typical asymmetric mass distribution and a very sharp symmetric one was clearly observed between $$^{256}$$Fm and $$^{258}$$Fm, while the spontaneous fission of $$^{259}$$Lr was found to exhibit mixture of three different fission modes.

Oral presentation

Spontaneous fission studies for neutron-rich Fm and Lr isotopes

Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi*; Tomitsuka, Tomohiro*; Chiera, N. M.*; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro*; Nishio, Katsuhisa; et al.

no journal, , 

We have studied spontaneous fission of neutron-rich Fm and Lr isotopes. The neutron-rich Fm isotopes were produced with the $$^{254}$$Es target and the $$^{18}$$O beam delivered by the JAEA tandem accelerator. The neutron-rich Lr isotope were produced with the $$^{248}$$Cm target and the $$^{15}$$N beam. Reaction products were mass-separated with an on-line isotope separator (ISOL), which enabled us to obtain non-contaminated samples and to measure fission fragments precisely. From the deduced fission-fragment mass and total kinetic energy distributions, we have obtained a new insight into the competition between the symmetric and asymmetric fission which is characteristic in this neutron-rich region.

Oral presentation

Depletion calculation of subcritical system with consideration of spontaneous fission reaction

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi

no journal, , 

Oral presentation

Measurement of spontaneous fission of Fm isotopes

Asai, Masato

no journal, , 

Fission-fragment mass distributions and total kinetic energy (TKE) distributions for the spontaneous fission of $$^{256}$$Fm, $$^{258}$$Fm, $$^{259}$$Md, and $$^{259}$$Lr have been measured precisely. These nuclei were produced in the multinucleon transfer reactions with the $$^{18}$$O beam and the $$^{254}$$Es target, and in the fusion-evaporation reaction of $$^{248}$$Cm($$^{15}$$N,4n)$$^{259}$$Lr at the JAEA tandem accelerator facility. The reaction products were mass-separated with the on-line isotope separator (ISOL), and the kinetic energies of spontaneous-fission fragments were measured with 4 pairs of Si semiconductor detectors. The results revealed that the three types of fission, the high-TKE and low-TKE symmetric fissions and asymmetric fission, compete or coexist in this neutron-rich Fm region.

Oral presentation

Measurement of mass and total kinetic energy distribution for spontaneous fission of $$^{259}$$Md

Asai, Masato; Ishibashi, Yuichi*; Tsukada, Kazuaki; Sato, Tetsuya; Aoki, Ryota*; Ito, Yuta; Uchibaba, Yuta*; Orlandi, R.; Gong, G.-M.*; Suzaki, Fumi; et al.

no journal, , 

Measurement of mass and total kinetic energy (TKE) distribution for the spontaneous fission (SF) of $$^{259}$$Md has been performed to clarify the fission mechanism in the neutron-rich fermium region. $$^{259}$$Md nuclei were produced with the $$^{254}$$Es target and $$^{18}$$O beam, and mass-separated with an on-line isotope separator (ISOL). We discuss the mechanism of fission observed in the SF of $$^{259}$$Md on the basis of the observed mass-TKE distribution.

Oral presentation

Symmetric fission properties of neutron-rich transfermium nuclei

Asai, Masato

no journal, , 

Symmetric fission properties of neutron-rich transfermium nuclei have been studied through the measurements of spontaneous fission fragments of $$^{258}$$Fm, $$^{259}$$Md, and $$^{259}$$Lr. These nuclei were produced in the multinucleon transfer reactions with the $$^{18}$$O beam and the $$^{254}$$Es target, and in the fusion-evaporation reaction of $$^{248}$$Cm($$^{15}$$N,4n)$$^{259}$$Lr at the JAEA tandem accelerator facility. The reaction products were mass-separated with the on-line isotope separator (ISOL), and the kinetic energies of spontaneous-fission fragments were measured with 4 pairs of Si semiconductor detectors. The deduced fission-fragment mass distributions and total kinetic energy distributions have revealed the detailed properties of symmetric fissions in this neutron-rich Fm and transfermium nuclei.

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